Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications

Zaid Alejandro Luzanilla Meléndrez; Alejandro Durán; Francisco Brown; Ofelia Hernández Negrete; Javier Hernández Paredes; Victor Emmanuel Alvarez Montano

doi:10.1007/978-3-031-22622-9_1

Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications

Zaid Alejandro Luzanilla Meléndrez, Alejandro Durán, Francisco Brown, Ofelia Hernández Negrete, Javier Hernández Paredes, Victor Emmanuel Alvarez Montano^*

^*Corresponding author for this work

Departamento de Ingeniería Química y Metalurgia

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

1 Scopus citations

Abstract

Indium Gallium Zinc Oxide (IGZO) is a ceramic material used in optoelectronic technology, having essential results such as high efficiency in energy consumption and better image quality in display devices. On the other hand, high-entropy ceramics (HECs) are an important route to design new and novel functional materials, and whose physical properties need to be explored. In this work, it is studied the HECs with IGZO-based compounds synthesized using conventional solid-state method. Several trivalent and divalent cations are substituted in the layered crystal structure of IGZO, and the equilibrium of phases is studied under different compositions and high temperatures. The classic quenching method is used, cooling in air from 1400 °C to room temperature. Phase equilibrium was monitored using X-ray powder diffractometry (XRD) and scanning electron microscopy (SEM) to reveal microstructure and cation distribution with elemental mapping. In addition, once the single phase with high-entropy composition is obtained, the dielectric properties are explored to analyze their possible electroceramic applications.

Original language	English
Title of host publication	Advances in Powder and Ceramic Materials Science 2023
Editors	Bowen Li, Dipankar Ghosh, Eugene A. Olevsky, Kathy Lu, Faqin Dong, Jinhong Li, Ruigang Wang, Alexander D. Dupuy, Elisa Torresani
Publisher	Springer Science and Business Media Deutschland GmbH
Pages	3-10
Number of pages	8
ISBN (Print)	9783031226212
DOIs	https://doi.org/10.1007/978-3-031-22622-9_1
State	Published - 2023
Event	Advances in Powder and Ceramic Materials Science Symposium, held at the TMS Annual Meeting and Exhibition, TMS 2023 - San Diego, United States Duration: 19 Mar 2023 → 23 Mar 2023

Publication series

Name	Minerals, Metals and Materials Series
ISSN (Print)	2367-1181
ISSN (Electronic)	2367-1696

Conference

Conference	Advances in Powder and Ceramic Materials Science Symposium, held at the TMS Annual Meeting and Exhibition, TMS 2023
Country/Territory	United States
City	San Diego
Period	19/03/23 → 23/03/23

Bibliographical note

Funding Information:
ZALM acknowledges the support from CONACyT for his graduate studies. AD and VEAM appreciate the support through the ‘Intercambio Académico’ program promoted by the Coordination of Scientific Research (CIC)-UNAM and the Universidad de Sonora.

Publisher Copyright:
© 2023, The Minerals, Metals & Materials Society.

Keywords

High entropy ceramics
IGZO
Phase equilibrium

Access to Document

10.1007/978-3-031-22622-9_1

Cite this

Luzanilla Meléndrez, Z. A., Durán, A., Brown, F., Hernández Negrete, O., Hernández Paredes, J., & Alvarez Montano, V. E. (2023). Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications. In B. Li, D. Ghosh, E. A. Olevsky, K. Lu, F. Dong, J. Li, R. Wang, A. D. Dupuy, & E. Torresani (Eds.), Advances in Powder and Ceramic Materials Science 2023 (pp. 3-10). (Minerals, Metals and Materials Series). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-031-22622-9_1

Luzanilla Meléndrez, Zaid Alejandro ; Durán, Alejandro ; Brown, Francisco et al. / Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications. Advances in Powder and Ceramic Materials Science 2023. editor / Bowen Li ; Dipankar Ghosh ; Eugene A. Olevsky ; Kathy Lu ; Faqin Dong ; Jinhong Li ; Ruigang Wang ; Alexander D. Dupuy ; Elisa Torresani. Springer Science and Business Media Deutschland GmbH, 2023. pp. 3-10 (Minerals, Metals and Materials Series).

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abstract = "Indium Gallium Zinc Oxide (IGZO) is a ceramic material used in optoelectronic technology, having essential results such as high efficiency in energy consumption and better image quality in display devices. On the other hand, high-entropy ceramics (HECs) are an important route to design new and novel functional materials, and whose physical properties need to be explored. In this work, it is studied the HECs with IGZO-based compounds synthesized using conventional solid-state method. Several trivalent and divalent cations are substituted in the layered crystal structure of IGZO, and the equilibrium of phases is studied under different compositions and high temperatures. The classic quenching method is used, cooling in air from 1400 °C to room temperature. Phase equilibrium was monitored using X-ray powder diffractometry (XRD) and scanning electron microscopy (SEM) to reveal microstructure and cation distribution with elemental mapping. In addition, once the single phase with high-entropy composition is obtained, the dielectric properties are explored to analyze their possible electroceramic applications.",

keywords = "High entropy ceramics, IGZO, Phase equilibrium",

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note = "Publisher Copyright: {\textcopyright} 2023, The Minerals, Metals & Materials Society.; Advances in Powder and Ceramic Materials Science Symposium, held at the TMS Annual Meeting and Exhibition, TMS 2023 ; Conference date: 19-03-2023 Through 23-03-2023",

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pages = "3--10",

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Luzanilla Meléndrez, ZA, Durán, A, Brown, F , Hernández Negrete, O , Hernández Paredes, J & Alvarez Montano, VE 2023, Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications. in B Li, D Ghosh, EA Olevsky, K Lu, F Dong, J Li, R Wang, AD Dupuy & E Torresani (eds), Advances in Powder and Ceramic Materials Science 2023. Minerals, Metals and Materials Series, Springer Science and Business Media Deutschland GmbH, pp. 3-10, Advances in Powder and Ceramic Materials Science Symposium, held at the TMS Annual Meeting and Exhibition, TMS 2023, San Diego, United States, 19/03/23. https://doi.org/10.1007/978-3-031-22622-9_1

Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications. / Luzanilla Meléndrez, Zaid Alejandro; Durán, Alejandro; Brown, Francisco et al.
Advances in Powder and Ceramic Materials Science 2023. ed. / Bowen Li; Dipankar Ghosh; Eugene A. Olevsky; Kathy Lu; Faqin Dong; Jinhong Li; Ruigang Wang; Alexander D. Dupuy; Elisa Torresani. Springer Science and Business Media Deutschland GmbH, 2023. p. 3-10 (Minerals, Metals and Materials Series).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications

AU - Luzanilla Meléndrez, Zaid Alejandro

AU - Durán, Alejandro

AU - Brown, Francisco

AU - Hernández Negrete, Ofelia

AU - Hernández Paredes, Javier

AU - Alvarez Montano, Victor Emmanuel

PY - 2023

Y1 - 2023

N2 - Indium Gallium Zinc Oxide (IGZO) is a ceramic material used in optoelectronic technology, having essential results such as high efficiency in energy consumption and better image quality in display devices. On the other hand, high-entropy ceramics (HECs) are an important route to design new and novel functional materials, and whose physical properties need to be explored. In this work, it is studied the HECs with IGZO-based compounds synthesized using conventional solid-state method. Several trivalent and divalent cations are substituted in the layered crystal structure of IGZO, and the equilibrium of phases is studied under different compositions and high temperatures. The classic quenching method is used, cooling in air from 1400 °C to room temperature. Phase equilibrium was monitored using X-ray powder diffractometry (XRD) and scanning electron microscopy (SEM) to reveal microstructure and cation distribution with elemental mapping. In addition, once the single phase with high-entropy composition is obtained, the dielectric properties are explored to analyze their possible electroceramic applications.

AB - Indium Gallium Zinc Oxide (IGZO) is a ceramic material used in optoelectronic technology, having essential results such as high efficiency in energy consumption and better image quality in display devices. On the other hand, high-entropy ceramics (HECs) are an important route to design new and novel functional materials, and whose physical properties need to be explored. In this work, it is studied the HECs with IGZO-based compounds synthesized using conventional solid-state method. Several trivalent and divalent cations are substituted in the layered crystal structure of IGZO, and the equilibrium of phases is studied under different compositions and high temperatures. The classic quenching method is used, cooling in air from 1400 °C to room temperature. Phase equilibrium was monitored using X-ray powder diffractometry (XRD) and scanning electron microscopy (SEM) to reveal microstructure and cation distribution with elemental mapping. In addition, once the single phase with high-entropy composition is obtained, the dielectric properties are explored to analyze their possible electroceramic applications.

KW - High entropy ceramics

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KW - Phase equilibrium

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DO - 10.1007/978-3-031-22622-9_1

M3 - Contribución a la conferencia

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SN - 9783031226212

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BT - Advances in Powder and Ceramic Materials Science 2023

A2 - Li, Bowen

A2 - Ghosh, Dipankar

A2 - Olevsky, Eugene A.

A2 - Lu, Kathy

A2 - Dong, Faqin

A2 - Li, Jinhong

A2 - Wang, Ruigang

A2 - Dupuy, Alexander D.

A2 - Torresani, Elisa

PB - Springer Science and Business Media Deutschland GmbH

T2 - Advances in Powder and Ceramic Materials Science Symposium, held at the TMS Annual Meeting and Exhibition, TMS 2023

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Luzanilla Meléndrez ZA, Durán A, Brown F , Hernández Negrete O , Hernández Paredes J , Alvarez Montano VE. Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications. In Li B, Ghosh D, Olevsky EA, Lu K, Dong F, Li J, Wang R, Dupuy AD, Torresani E, editors, Advances in Powder and Ceramic Materials Science 2023. Springer Science and Business Media Deutschland GmbH. 2023. p. 3-10. (Minerals, Metals and Materials Series). doi: 10.1007/978-3-031-22622-9_1

Design of High-Entropy Ceramics with IGZO-Based Compounds for Electroceramics Applications

Abstract

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Bibliographical note

Keywords

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